杩戞棩锛屽寲瀛︿笌鏉愭枡绉戝瀛﹂櫌鍒嗘瀽绉戝鎶€鏈鐮斿洟闃熷湪绾崇背浼犳劅鍣ㄧ爺绌堕鍩熷彇寰楃郴鍒楅噸瑕佽繘灞曪紝鐩稿叧鐮旂┒鎴愭灉杩炵画鍙戣〃鍦ㄥ浗闄呯煡鍚嶆湡鍒娿€夾nalytical Chemistry銆嬨€侟/p>
锛?锛堻/strong>浠ラ噾灞?鏈夋満妗嗘灦绾崇背棰楃矑锛圡OFs锛堻/strong>涓烘棤鏍囪鑽у厜鏍囩鍩轰簬鍏夊彲鎺NA Walker鍒嗗瓙鐢佃矾鐢?/strong>浜嶞/strong>MicroRNA-21鐨勫彲璋冭皭妫€娴婞/strong>
璇ュ洟闃熷熀浜嶮OFs锛圲iO-66-NH2锛夌殑纾烽吀婵€娲荤壒鎬у強鍏朵笌Zr鍘熷瓙鐨勭珵浜夋€ч厤浣嶄綔鐢紝缁撳悎閭荤鍩鸿媱鍩虹殑鍏夊彲鎺ф€ц川鍜孌NA walker浼犳劅鍣紝浠iO-66-NH2浣滀负鏃犳爣璁拌崸鍏夋爣绛撅紝鏋勫缓浜唌iR-21鍙皟璋愯崸鍏変紶鎰熷櫒銆傛娴嬪姩鎬佽寖鍥村彲浠ョ簿纭湴浠?00鍊嶈皟鑺傚埌67000鍊嶏紝妫€娴嬭寖鍥翠粠2.5 fM鍒?6.7 pM鍙皟锛屽悓鏃堕伩鍏嶄簡鏍囪鐗╁鎺㈤拡鎬ц川鐨勬綔鍦ㄥ共鎵般€傛湰鐮旂┒涓轰复搴婃牱鏈腑鐨勯€昏緫璁＄畻鍜岀檶鐥囪瘖鏂瀯寤轰簡甯冨皵閫昏緫鏍戝拰澶嶆潅鍒嗗瓙鐢佃矾锛屼负澶嶆潅鐢熺墿浼犳劅绯荤粺杞寲涓哄彲鎿嶄綔鐨勫尰鐤楀喅绛栨彁渚涗簡寮哄ぇ瑙ｅ喅鏂规锛屾湁鍔╀簬鐤剧梾鏃╂湡璇婃柇銆傜浉鍏虫垚鏋溾€淧hotocontrollable DNA Walker-Based Molecular Circuit for the Tunable Detection of MicroRNA-21 Using Metal鈭扥rganic Frameworks as Label-Free Fluorescence Tags鈥濆彂琛ㄥ湪Analytical Chemistry锛?023, DOI: 10.1021/acs.analchem.3c03913锛夛紝钁ｆ睙闆壇鏁欐巿涓虹涓€浣滆€咃紝娴庡崡澶у楂樹腑閿嬪壇鏁欐巿涓洪€氳浣滆€咃紝娌冲寳澶у涓虹涓€瀹屾垚鍗曚綅銆侟/p>
锛?锛変互D-闈掗湁鑳篅Ag/Cu绾崇背绨嘃/strong>锛圏/strong>DPA@Ag/Cu NCs锛堻/strong>涓烘帰閽堢敤浜庣瓫閫夌７閰搁叝绫绘湁鏈虹７鍐滆嵂鍜岄€昏緫淇℃伅鍔犲瘑
璇ュ洟闃熶互璇鹃缁勫埗澶囩殑榛勮壊鑽у厜DPA@Ag/Cu NCs涓烘帰閽堬紝瀹炵幇浜嗕粠甯歌鏈夋満纾峰啘鑽腑绛涢€塐OPs锛屽悇鏈夋満纾峰鑷寸殑鑽у厜淇″彿鍙樺寲瓒嬪娍涓庣悊璁鸿绠楃殑鍒嗗瓙鐢佃礋鎬х粨鏋滀竴鑷淬€傚熀浜庝笂杩颁紶鎰熶綋绯伙紝鎴愬姛璁捐浜咲PA@Ag/Cu NCs閫昏緫浼犳劅绯荤粺锛屾瀯寤轰簡鍏锋湁澶嶆潅閫昏緫鐢佃矾鐨勫垎瀛愯绠楀竷灏旈€昏緫鏍戙€傞€氳繃瀵规湁鏈虹７鍐滆嵂鐨勮崸鍏夊搷搴旇繘琛屾彁鍙栧拰浜岃繘鍒惰浆鎹紝寮€鍙戜簡涓€绉嶇敤浜庡姞瀵嗙壒瀹氫俊鎭殑浜哄伐鑽у厜绾崇背绁炵粡鍏冿紝瀹炵幇浜嗗垎瀛愯绠椼€佺紪鐮併€佸瓨鍌ㄥ拰淇℃伅鍔犲瘑銆傜浉鍏虫垚鏋溾€淒鈥慞enicillamine@Ag/Cu Nanocluster-Based Fluorescent Nanoneuron for Logic Screening Phosphonate-Type Organophosphate Pesticides and Steganographically Encrypting Information鈥濆彂琛ㄥ湪Analytical Chemistry锛?023锛?5锛?1113锛夛紝鍖栧闄㈠崥澹敓鑼冧簹鏉颁负绗竴浣滆€咃紝钁ｆ睙闆壇鏁欐巿銆佺敵涓栧垰鏁欐巿鍜屾祹鍗楀ぇ瀛﹂珮涓攱鍓暀鎺堜负鍏卞悓閫氳浣滆€咃紝娌冲寳澶у涓虹涓€瀹屾垚鍗曚綅銆侟/p>
浠ヤ笂鐮旂┒宸ヤ綔寰楀埌浜嗘渤鍖楃渷鑷劧绉戝鍩洪噾銆佹渤鍖楀ぇ瀛︾鐮斿垱鏂板洟闃熴€佹渤鍖楃渷閲嶇偣涓撻」绛夐」鐩殑璧勫姪鍜屾敮鎸併€侟/p>